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Mundo hands down. His Q would eat singed alive. Singed has amazing health and speed, but with mundo passive and his ult he would regen almost all of his health. He could then just spam Q to own singed. Since it works off singed, mundo is the true counter to champions like singed. Including ramnus and others.
Mundo practically has 140% health including ult cost. They both do good damage. At the same level of tankiness, then Mundo would win.